B. M. Tanygin, V. F. Kovalenko, M. V. Petrychuk, S. A. Dzyan
Investigations of the phase transitions and self-organization in the magnetic aggregates are of the fundamental and applied interest. The long-range ordering structures described in the Tom\'anek's systematization (M. Yoon, and D. Tom\'anek, 2010 [1]) are not yet obtained in the direct molecular dynamics simulations. The resulted structures usually are the linear chains or circles, or, else, amorphous (liquid) formations. In the present work, it was shown, that the thermodynamically equilibrium primary ferrofluid aggregate has either the long-range ordered or liquid phase. Due to the unknown steric layer force and other model idealizations, the clear experimental verification of the real equilibrium phase is still required. The predicted long-range ordered (crystallized) phase produces the faceting shape of the primary ferrofluid aggregate, which can be recognized experimentally. The medical (antiviral) application of the crystallized aggregates has been suggested. Dynamic formation of all observed ferrofluid nanostructures conforms to the Tom\'anek's systematization.
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http://arxiv.org/abs/1112.4431
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