1202.4319 (D. Choudhury et al.)

Near room-temperature colossal magnetodielectricity and multiglass
properties in partially-disordered La2NiMnO6    [PDF]

D. Choudhury, P. Mandal, R. Mathieu, A. Hazarika, S. Rajan, A. Sundaresan, U. V. Waghmare, R. Knut, O. Karis, P. Nordblad, D. D. Sarma

We report magnetic, dielectric and magnetodielectric responses of pure
monoclinic bulk phase of partially-disordered La2NiMnO6, exhibiting a spectrum
of unusual properties and establish that this system intrinsically is a true
multiglass with a large magnetodielectric coupling (8-20%) over a wide range of
temperatures (150 - 300 K). Specifically, our results establish a unique way to
obtain colossal magnetodielectricity, independent of any striction effects, by
engineering the asymmetric hopping contribution to the dielectric constant via
the tuning of the relative spin orientations between neighboring magnetic ions
in a transition metal oxide system. We discuss the role of anti-site (Ni-Mn)
disorder in emergence of these unusual properties.

View original: http://arxiv.org/abs/1202.4319